The focus of environmental ethics should indeed be on the virtues and how these inform our relationship to natural environments.
Gardening is an excellent example of a practice to which, as Alasdair MacIntyre puts it, certain virtues are 'internal'. Good gardening requires a certain goodness on the part of the gardener: care, humility, patience, and respect, for example.
Chuang Tzu and Heidegger both emphasise the virtue of 'spontaneity' - a sort of mindful responsiveness to things as they are. It's this notion, I suspect, that is the best bet for helping to make some sense of talk about harmony or unity with nature.
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